MacFarlane, D. R., Newman, P. J., Nairn, K. M. and Forsyth, M. 1998, Lithium-ion conducting ceramic/polyether composites, Electrochimica acta, vol. 43, no. 10-11, pp. 1333-1337, doi: 10.1016/S0013-4686(97)10039-1.
Composites of a lithium ion conducting ceramic with a lithium salt based polymer electrolyte matrix are described. Conductivity measurements as a function of the lithium ion conducting ceramic phase content in the composite show that there is a significant increase in conductivity at approximately 40 vol% of the ceramic. The room temperature conductivity above this ceramic content is enhanced by at least 100% over that of the polymer electrolyte phase alone. It is believed that this additional contribution is substantially lithium ion conduction. The major barrier to ion-motion in these materials appears to be the interface between the polymer and ceramic. This interfacial resistance is strongly moisture-sensitive.
Field of Research
039999 Chemical Sciences not elsewhere classified
Socio Economic Objective
970103 Expanding Knowledge in the Chemical Sciences
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