Simultaneously 'pushing' and 'pulling' graphene oxide into low-polar solvents through a designed interface

Liu, Zhen, Liu, Jingquan, Wang, Yichao, Razal, Joselito M., Francis, Paul S., Biggs, Mark J., Barrow, Colin J. and Yang, Wenrong 2018, Simultaneously 'pushing' and 'pulling' graphene oxide into low-polar solvents through a designed interface, Nanotechnology, vol. 29, no. 31, pp. 1-9, doi: 10.1088/1361-6528/aac455.

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Title Simultaneously 'pushing' and 'pulling' graphene oxide into low-polar solvents through a designed interface
Author(s) Liu, Zhen
Liu, Jingquan
Wang, Yichao
Razal, Joselito M.ORCID iD for Razal, Joselito M. orcid.org/0000-0002-9758-3702
Francis, Paul S.ORCID iD for Francis, Paul S. orcid.org/0000-0003-4165-6922
Biggs, Mark J.
Barrow, Colin J.ORCID iD for Barrow, Colin J. orcid.org/0000-0002-2153-7267
Yang, WenrongORCID iD for Yang, Wenrong orcid.org/0000-0001-8815-1951
Journal name Nanotechnology
Volume number 29
Issue number 31
Article ID 315707
Start page 1
End page 9
Total pages 9
Publisher IOPSCience
Place of publication Bristol, Eng.
Publication date 2018-06
ISSN 1361-6528
Keyword(s) graphene oxide
interface design
phase transfer
self-assembly
surface chemistry
Summary Dispersing graphene oxide (GO) in low-polar solvents can realize a perfect self-assembly with functional molecules and application in removal of organic impurities that only dissolve in low-polar solvents. The surface chemistry of GO plays an important role in its dispersity in these solvents. The direct transfer of hydrophilic GO into low-polar solvents, however, has remained an experimental challenge. In this study, we design an interface to transfer GO by simultaneously "pushing and pulling" the nanosheets into low-polar solvents. Our approach is outstanding due to the ability to obtain monolayers of chemically reduced GO (CRGO) with designed surface properties in the organic phase. Using the transferred GO or CRGO dispersions, we have fabricated GO/fullerene nanocomposites and assessed the ability of CRGOs for dye adsorption. We hope our work can provide a universal approach for the phase transfer of other nanomaterials.
Language eng
DOI 10.1088/1361-6528/aac455
Field of Research MD Multidisciplinary
HERDC Research category C1 Refereed article in a scholarly journal
ERA Research output type C Journal article
Copyright notice ©2018, IOP Publishing
Persistent URL http://hdl.handle.net/10536/DRO/DU:30108435

Document type: Journal Article
Collection: School of Life and Environmental Sciences
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