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Polymeric ionic liquids for lithium-based rechargeable batteries
journal contribution
posted on 2019-01-01, 00:00 authored by G G Eshetu, D Mecerreyes, Maria ForsythMaria Forsyth, H Zhang, M ArmandThe quest for reliable and high-performance batteries has incentivized the development of new battery chemistries/materials that can potentially improve the current lithium-ion battery technologies in terms of gravimetric/volumetric energy density and safety. Polymeric ionic liquids containing both ionic liquid-like moieties and polymer frameworks are emerging as alternative electrolyte/binder candidates for Li-based rechargeable batteries, owing to their various intrinsic features, such as superior mechanical and chemical stability, structural controllability over the IL species and macromolecular backbone and leak-proof nature and thereby improved safety. In this perspective, recent progress and advances on the use of PIL-based electrolytes and binders for Li-based rechargeable batteries are overviewed and discussed, with particular focus on the structural-property relationships. Future directions and improvements of the properties of PIL-based materials are given from the standpoint of chemistry of Li-based batteries.
History
Journal
Molecular Systems Design and EngineeringVolume
4Issue
2Pagination
294 - 309Publisher
Royal Society of ChemistryLocation
London, Eng.Publisher DOI
eISSN
2058-9689Language
engPublication classification
C1 Refereed article in a scholarly journalCopyright notice
2019, The Royal Society of ChemistryUsage metrics
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No categories selectedKeywords
Science & TechnologyPhysical SciencesTechnologyChemistry, PhysicalEngineering, ChemicalNanoscience & NanotechnologyMaterials Science, MultidisciplinaryChemistryEngineeringScience & Technology - Other TopicsMaterials ScienceSOLID-STATE ELECTROLYTESPOLY(IONIC LIQUID)ELECTROCHEMICAL PROPERTIESPOLYELECTROLYTE SOLUTIONSELECTRICAL-CONDUCTIVITYCOUNTERION CONDENSATIONINTERFACIAL PROPERTIESTRANSPORT MECHANISMMOLECULAR-WEIGHTGEL ELECTROLYTE
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